Yeah, I have a few large cylinders of pure Argon for TIG welding,
and debated on using it in pcp rifles too, but all I could find was that it is a heavier gas..
That said, it would not be very efficient. Especially compared to Nitrogen and Helium.
Helium though is a Non Renewable gas, so once it's gone, it's gone for good..
They've already started to restrict it..
Nitrogen - Probably the best bet for PCP refilling.
Sam -